Physical mixing of metal acetates: Optimisation of catalyst parameters to produce highly active bimetallic catalysts

Peter J. Miedziak, Simon A. Kondrat, Noreen Sajjad, Gavin M. King, Mark Douthwaite, Greg Shaw, Gemma L. Brett, Jennifer K. Edwards, David J. Morgan, Ghulam Hussain, Graham J. Hutchings*

*Awdur cyfatebol y gwaith hwn

Allbwn ymchwil: Cyfraniad at gyfnodolynErthygladolygiad gan gymheiriaid

3 Dyfyniadau (Scopus)

Crynodeb

We have investigated the optimisation of the catalytic parameters for the preparation of catalysts by the simple mixing and thermal treatment of a support and metal acetate precursors. We have studied the effect of metal ratio and metal loading to produce a catalyst which has the optimum activity for a variety of reactions including benzyl alcohol oxidation, glycerol oxidation and the direct synthesis of hydrogen peroxide. We have demonstrated the high activity of these catalyst's for a variety of substrates and performed XPS and XRD studies on the catalysts to help elucidate the origin of the catalysts improved activity.

Iaith wreiddiolSaesneg
Tudalennau (o-i)2910-2917
Nifer y tudalennau8
CyfnodolynCatalysis Science and Technology
Cyfrol3
Rhif cyhoeddi11
Dynodwyr Gwrthrych Digidol (DOIs)
StatwsCyhoeddwyd - 1 Hyd 2013
Cyhoeddwyd yn allanolIe

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