Gold-palladium core-shell nanocrystals with size and shape control optimized for catalytic performance

Anna M. Henning; John Watt; Peter J. Miedziak; Soshan Cheong; Marco Santonastaso; Minghui Song; Yoshihiko Takeda; Angus I. Kirkland; Stuart H. Taylor; Richard D. Tilley

doi:10.1002/anie.201207824

Gold-palladium core-shell nanocrystals with size and shape control optimized for catalytic performance

Anna M. Henning, John Watt, Peter J. Miedziak, Soshan Cheong, Marco Santonastaso, Minghui Song, Yoshihiko Takeda, Angus I. Kirkland, Stuart H. Taylor, Richard D. Tilley^*

^*Awdur cyfatebol y gwaith hwn

Allbwn ymchwil: Cyfraniad at gyfnodolyn › Erthygl › adolygiad gan gymheiriaid

66 Dyfyniadau (Scopus)

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Right to the core: The design of nanocatalysts with maximized catalytic performance relies on control of the size, shape, and composition. The shell thickness of nanocrystals with core-shell structures can be controlled, thus enabling control over the nanocrystal electronic structure and catalytic properties. Monodisperse faceted icosahedral Au-Pd core-shell nanocrystals (see picture) were synthesized, and optimized for the oxidation of benzyl alcohol to benzaldehyde.

Iaith wreiddiol	Saesneg
Tudalennau (o-i)	1477-1480
Nifer y tudalennau	4
Cyfnodolyn	Angewandte Chemie - International Edition
Cyfrol	52
Rhif cyhoeddi	5
Dynodwyr Gwrthrych Digidol (DOIs)	https://doi.org/10.1002/anie.201207824
Statws	Cyhoeddwyd - 28 Ion 2013
Cyhoeddwyd yn allanol	Ie

Mynediad at Ddogfen

10.1002/anie.201207824Trwydded: CC BY-NC-ND

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@article{87a5a7fe3480432a9e6af046c64a9e6f,

title = "Gold-palladium core-shell nanocrystals with size and shape control optimized for catalytic performance",

abstract = "Right to the core: The design of nanocatalysts with maximized catalytic performance relies on control of the size, shape, and composition. The shell thickness of nanocrystals with core-shell structures can be controlled, thus enabling control over the nanocrystal electronic structure and catalytic properties. Monodisperse faceted icosahedral Au-Pd core-shell nanocrystals (see picture) were synthesized, and optimized for the oxidation of benzyl alcohol to benzaldehyde.",

keywords = "bimetallic nanoparticles, core-shell structures, gold, heterogeneous catalysis, palladium",

author = "Henning, {Anna M.} and John Watt and Miedziak, {Peter J.} and Soshan Cheong and Marco Santonastaso and Minghui Song and Yoshihiko Takeda and Kirkland, {Angus I.} and Taylor, {Stuart H.} and Tilley, {Richard D.}",

year = "2013",

month = jan,

day = "28",

doi = "10.1002/anie.201207824",

language = "English",

volume = "52",

pages = "1477--1480",

journal = "Angewandte Chemie International Edition",

issn = "1433-7851",

publisher = "Wiley",

number = "5",

}

TY - JOUR

T1 - Gold-palladium core-shell nanocrystals with size and shape control optimized for catalytic performance

AU - Henning, Anna M.

AU - Watt, John

AU - Miedziak, Peter J.

AU - Cheong, Soshan

AU - Santonastaso, Marco

AU - Song, Minghui

AU - Takeda, Yoshihiko

AU - Kirkland, Angus I.

AU - Taylor, Stuart H.

AU - Tilley, Richard D.

PY - 2013/1/28

Y1 - 2013/1/28

N2 - Right to the core: The design of nanocatalysts with maximized catalytic performance relies on control of the size, shape, and composition. The shell thickness of nanocrystals with core-shell structures can be controlled, thus enabling control over the nanocrystal electronic structure and catalytic properties. Monodisperse faceted icosahedral Au-Pd core-shell nanocrystals (see picture) were synthesized, and optimized for the oxidation of benzyl alcohol to benzaldehyde.

AB - Right to the core: The design of nanocatalysts with maximized catalytic performance relies on control of the size, shape, and composition. The shell thickness of nanocrystals with core-shell structures can be controlled, thus enabling control over the nanocrystal electronic structure and catalytic properties. Monodisperse faceted icosahedral Au-Pd core-shell nanocrystals (see picture) were synthesized, and optimized for the oxidation of benzyl alcohol to benzaldehyde.

KW - bimetallic nanoparticles

KW - core-shell structures

KW - gold

KW - heterogeneous catalysis

KW - palladium

U2 - 10.1002/anie.201207824

DO - 10.1002/anie.201207824

M3 - Article

AN - SCOPUS:84872845532

VL - 52

SP - 1477

EP - 1480

JO - Angewandte Chemie International Edition

JF - Angewandte Chemie International Edition

SN - 1433-7851

IS - 5

ER -

Gold-palladium core-shell nanocrystals with size and shape control optimized for catalytic performance

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